I'd say go with the 072. Depending on what equipment you are running, you can get some pretty substantial overhangs on the curves. 0-63 and STD-57 only gives you 3" between tracks on a concentric curve - that's not enough. The larger gap between the two different size tracks will be better visually - having the large and small trains cramped together won't look good. And finally, 0-72 gives you more flexibility in what you can run on the 0 gauge loop. Bigger is always better when it comes to curve diameter.
I am running STD-87 (also from USA Track) on the outside of an 0 gauge layout with 0-72 curves. There's enough distance between the tracks, and I wouldn't want them any closer. Here's my layout. The curve sizes are STD-87, 0-72, 0-63, and 0-42. As you can see, there's not a lot of room between the 87" and 72" lines. If I pulled up the 0-42 and tried to lay STD-57 inside the 0-63, it wouldn't work.
And finally, here's a reference shot of all the 0 gauge tubular sizes from 0-31 to 0-72. From inside to outside: 0-31, 0-42, 0-54. 0-63, 0-72. I made this photo when I was laying out my track, to help me decide on my curve diameters. I think you will see from the relationship between 0-54 and 0-63 that STD-57 and 0-63 wouldn't work well with concentric (parallel) curves. Click on the photos for a larger image.