The Lionel KW is certainly one of the well regarded transformers of the post war era. They are readily available and prices seem to have come down in recent years. It is worth considering why KWs and other post war transformers are not as hotly sought after as they were through the 1990s.
John and Dale have both mentioned considerations that come with the use of a post war transformer for modern trains. If you use one it is prudent to add extra protection for the trains with modern breakers and/or transient voltage suppressors.
I think it is also worth considering the type of duty you are asking a 50 or 60 year old transformer to perform. Do you really want to rely on such an old electrical device 42 hours a week?
KWs are relatively inexpensive now due in part to the fact that we have had several modern alternatives for over a decade now. Today the Z-4000 is the benchmark large transformer and the Z-1000 sets the standard for train set transformers. They come out of the box with modern circuit protection and a UL listing.
If you knew a young couple who was getting married would you consider giving them a 60 year old toaster as a wedding gift? Why use a 60 year old electrical appliance for a high duty cycle application in a children's museum?
If you are running modern trains and have a modern power supply you will have some good options to add play value for the kids. You could stick with conventional control but give access to a bell and whistle button. Command equipped locomotives could be operated in conventional mode on the museum layout but be preset with sound settings limited to appropriate levels for the environment.
If you make the jump to command more options open up. One area super market has a display layout that operates periodically according to a set command control program. And the Edmonds Historical Museum has the Pacific Fast Mail display layout and now operates Proto 3 locomotives on it with the DCS remote commander. The sound makes that a big hit with kids of all ages.