I've done three conversions on Lionel "traditional" F-3s from the MPC and the LTI era, primarily to convert them so they were TMCC and Railsounds equipped. I used chassis' from PWC F-3s, which were equipped with TMCC, R/S, finished interiors, directional lighting, and electrocouplers. Swapping shells is pretty easy, as is mounting the TMCC antenna in the old shell. However, mounting the older shell on the Railsounds-equipped chassis (I've done this with both B and A units) is more challenging, and required some surgery to install the speaker in the roof, install the volume control, etc., but that's another story.
In any case, if the chassis' on your engines were completely black, you'd have several routes you could go. However, your options with these particular Northern Pacific engines are limited, because, as has been noted, part of the frame sides, the fuel tank, and (on the A) the pilot are all painted green. Theoretically, it would be possible to paint these, but I won't attempt it. It would be very difficult to achieve a perfect match, and getting a smooth application, unless you could figure out how to spray it on, would be extremely difficult as well.
By far the simplist solution, and what I would do, is just buy another A-B set, and use the powered A in your consist along with your current powered A and B unit (which has the RailSounds, of course). You could also then run ABBA of course, or ABB (which can look pretty cool, incidently), or just sell the extra B unit. Before you sell the extra B, though, you should check out what the sounds are like with two RailSounds engines operating at the same time.