Test results:
I was able to find the 208/240V leads. I applied 120V to the 208 tap.
The other two (identical) windings give me "off-center tapped" windings with 49.8V on one half and 18.6V on the other half. The 18.6V would be pretty good for running trains.
How much current is available? I don't know, but the wires are #8AWG, and there are two coils available. I would guess at least 60-80 amps, and I wouldn't expect much voltage sag under load. This device was originally intended for 208/240V operation, which means when I use it for 120V operation I have more copper in the circuit than is necessary, but my guess is that the copper is so big that it wouldn't be much of a penalty for this application.
The core magnetizing (no-load idling) current draws only 15VA and 9 watts. The toroidal core is very efficient. In comparison, a Lionel 180 watt brick draws 36VA and 4 watts idling.
Actually, I wouldn't want to try this on a layout. The instantaneous current during a derail, before the circuit breaker or fuse can act, would be sky high, welding everything in sight!